рус eng
«IZVESTIYA IRKUTSKOGO GOSUDARSTVENNOGO UNIVERSITETA». SERIYA «NAUKI O ZEMLE»
«THE BULLETIN OF IRKUTSK STATE UNIVERSITY». SERIES «EARTH SCIENCES»
ISSN 2073-3402 (Print)

List of issues > Series «Earth Sciences». 2018. Vol. 24

Ozone and Oxides of Sulfur and Nitrogen in the Near-Surface Atmosphere above the Baikal Natural Territory

Author(s)
O. I. Khuriganova, V. A. Obolkin, V. L. Potemkin, L. P. Golobokova, T. V. Khodzher
Abstract
Spatial and time dynamics of concentrations of the major gaseous impurities (O3, SO2 and NOx) were studied in 2015-2016 at three monitoring sites located on the Baikal Natural Territory (BNT) in the south of East Siberia. The authors used passive (diffusive), forced (filtration) and direct (gas analyzers) methods in the investigations with the correlation of 0.7 and higher.
The results obtained confirmed patterns of annual trends in the ozone distribution in the near-surface atmosphere at monitoring sites: maximal concentrations in spring (March-April) and minimal values in autumn (September-October). Mean concentrations of ozone were substantially lower at the urban site Irkutsk than at background site Mondy and rural site Listvyanka. Short-term fluctuations of ozone concentrations under urban conditions depended on the concentrations of sulfur and nitrogen oxides of anthropogenic character contrary to the background areas, where ozone concentrations were high during a year. The concentrations of sulfur and nitrogen dioxide in the urban and rural areas subjected significantly to seasonal and inter-annual fluctuations depending on air temperature varying during a year (in winter they were higher and in summer lower) and from year to year (in cold years higher and in warm years lower). At the site Listvyanka, the elevated concentrations of these gases were also recorded in the warm period. This is attributed to high recreational load of the settlement of Listvyanka as one of the largest tourist areas at Lake Baikal in the Irkutsk region.
For citation:
Khuriganova O. I., Obolkin V. A., Potemkin V. L., Golobokova L. P., Khodzher T. V. Ozone and Oxides of Sulfur and Nitrogen in the Near-Surface Atmosphere above the Baikal Natural Territory. The Bulletin of Irkutsk State University. Series Earth Sciences, 2018, vol. 24, pp. 111-123. https://doi.org/10.26516/2073-3402.2018.24.111. (in Russian)
Keywords
ozone, gas impurities, measurement methods, monitoring sites, atmosphere
UDC
551.510.41(571.5)

DOI

https://doi.org/10.26516/2073-3402.2018.24.111

References

Kotel'nikov S.N., Stepanov E.V., Shherbakov I.A., Ivashkin V.T. Aktualnost problemy troposfernogo ozona v Rossii [An importance of the tropospheric ozone problem for Russia]. Rossijskaja Akademija Nauk. Trudy instituta obshhej fiziki im. A.M. Prohorova [Prokhorov General Physics Institute of RAS], 2015, vol. 71, pp. 3-9. (in Russian).

Belan B.D. Ozon v troposfere [Ozone in the troposphere]. Tomsk, Institute of atmospheric optics SB RAS Publ., 2010, 488 p. (in Russian).

Belan B.D., Savkin D.E., Tolmachev G.N. Zavisimost obrazovaniya ozona v prizemnom sloe ot temperatury vozduha [Generation of ozone in the surface air layer versus air temperature]. Optika atmosf. i okeana [Atmospheric and oceanic optics], 2017, vol. 30, no. 11, pp. 971-979. DOI: 10.15372/AOO20171110. (in Russian).

Zvjagincev A.M., Kakadzhanova G., Tarasova O.A. Izmenchivost' prizemnogo ozona i drugih malyh gazovyh sostavljajushhih atmosfery v megapolise i sel'skoj mestnosti [Cycles of surface ozone and other trace gases in urban and rural regions]. Optika atmosferi i okeana [Atmospheric and oceanic optics], 2010, vol. 23, no. 1, pp. 32-37. (in Russian).

Holjavickaja A.A., Potjomkin V.L., Golobokova L.P., Hodzher T.V. Izmerenija koncentracii prizemnogo ozona passivnym metodom [Testing of the passive method for measuring ozone concentrations in the atmospheric surface layer (Mondy station, East Siberia)]. Optika atmosferi i okeana [Atmospheric and oceanic optics], 2011, vol. 24, no. 9, pp. 828-831. (in Russian).

Potemkin V.L., Latysheva I.V., Makuhin V.L., Hodzher T.V. Issledovanie processov rasprostranenija dioksida sery i ozona na juge Vostochnoj Sibiri [Studies of the dispersal of sulfur dioxide and ozone in the south of Eastern Siberia]. Optika atmosferi i okeana [Atmospheric and oceanic optics], 2006, vol. 19, no. 7, pp. 567-569. (in Russian).

Huriganova O.I., Obolkin V.A., Potemkin V.L., Hodzher T.V., Artem'eva O.V., Golobokova L.P. Koncentracii ozona v prizemnom sloe troposfery v urbanizirovannyh, sel'skih i fonovyh rajonah juga Vostochnoj Sibiri [Ozone concentration in the ground atmospheric layer in urban, rural, and background areas of the south of Eastern Siberia]. Optika atmosferi i okeana [Atmospheric and oceanic optics], 2015, vol. 28, no. 6, pp. 579-584. DOI: 10.15372/AOO20150614. (in Russian).

Kotel'nikov S.N. Osnovnye mehanizmy vzaimodejstvija ozona s zhivymi sistemami i osobennostjami problemy prizemnogo ozona dlya Rossii [The basic mechanisms of interaction of ozone with live systems and features of a problem of ground ozone for Russia]. Rossijskaya Akademija Nauk. Trudy instituta obshhej fiziki im. A.M. Prohorova [Prokhorov General Physics Institute of RAS], 2015, vol. 71, pp. 10-41. (in Russian).

Pankratova N.V., Elanskij N.F., Belikov I.B., Lavrova O.V., Skorohod A.I., Shumskij R.A. Ozon i okisly azota v prizemnom vozduhe Severnoj Evrazii po nabljudenijam v jeksperimentah TROICA [Ozone and Nitric Oxides in the Surface Air over Northern Eurasia According to Observational Data Obtained in TROICA Experiments]. Izvestija RAN. Fizika atmosfery i okeana [Izvestiya, Atmospheric and Oceanic Physics]. 2011, vol. 47, no. 3, pp. 343-358. (in Russian).

Akimoto H. Tropospheric Ozone a Growing Threat. Japan, Niigata, Acid deposition and oxidant research center Publ., 2006, 26 p.

Karagulian F., Belis C.A., Dora C.F.C., Prüss-Ustün A.M., Bonjour S., Adair-Rohani H., Amann M. Contributions to Cities' Ambient Particulate Matter (PM): A Systematic Review of Local Source Contributions at Global Level. Atmos. Environ, 2015, vol. 120, pp. 475-483. DOI: 10.1016/j.atmosenv.2015.08.087.

Kelly F.J., Fussell J.C. Size, Source and Chemical Composition as Determinants of Toxicity Attributable to Ambient Particulate Matter. Atmos. Environ, 2012, vol. 60, pp. 504-526. DOI: 10.1016/j.atmosenv.2012.06.039.

Lin C.C.-Y., Jacob D.J., Munger W., Fiore A.M. Increasing Background Ozone in Surface air Over the United States. Geophys. Res. Lett, 2000, vol. 27(21), pp. 3465-3468.

Lin J.-T., Patten K.O. Effects of Future Climate and Biogenic Emissions Changes on Surface Ozone over the United States and China. J. Appl. Meteorol. Climatol, 2007, vol. 47, pp. 1888-1909. DOI: 10.1175/2007JAMC1681.1.

Pochanart P., Akimoto H., Kajii Y., Potemkin V., Khodzher T. Regional Background Ozone and Carbon Monoxide Variations in Remote Siberia (East Asia). J. Geophys. Res, 2003, vol. 108(1), pp. ACH. 7-1-7-18. DOI: 10.1029/2001JD001412.

Pochanart P., Kato S., Katsuno T., Akimoto H. Eurasian Continental Background and Regionally Polluted Levels of Ozone and CO Observed in Northeast Asia. Atmos. Environ, 2004, vol. 38(9), pp. 1325-1336. DOI: 10.1016/j.atmosenv.2003.11.014.

Sahu S.K., Beig G. Parkhi N. Critical Emissions from the Largest On-Road Transport Network in South Asia. Aerosol and Air Qual Res, 2014, pp. 135-144. DOI: 10.4209/aaqr.2013.04.0137.

Vu T.V., Delgado-Saborit J.M., Harrison R.M. Review: Particle Number Size Distributions from Seven Major Sources and Implications for Source Apportionment Studies. Atmos. Environ, 2015, vol. 122, pp. 114-132. DOI: 10.1016/j.atmosenv.2015.09.027.


Full text (russian)